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Summary
Summary
A timely addition to the highly acclaimed four-volume handbook set; volumes 5 and 6 highlight recent developments, particularly in the fields of new materials, molecular modeling and durability.
Since the publication of the first four volumes of the Handbook of Fuel Cells in 2003, the focus of fuel cell research and development has shifted from optimizing fuel cell performance with well-known materials to developing new materials concepts, and to understanding the origins of materials and fuel cell degradation. This new two-volume set provides an authoritative and timely guide to these recent developments in fuel cell research.
Author Notes
Wolf Vielstich started research work on Fuel Fells and Fischer-Tropsch Synthesis at Ruhrchemie / Oberhausen. Working in the field of Fundamental and Applied Electrochemistry at the Institute of Physical Chemistry of Bonn University, he completed his Habilitation in Physical Chemistry in 1962. From 1965 he was a professor and director at the Bonn Institute. His special interest was new experimental methods like Rotating Ring Electrodes, online MS, Insitu IR and UHV-analysis of electrode surfaces, as well as to Batteries and Fuel Cells. His work in Electrochemistry has resulted in more than 250 publications, over 10 patents, books on Fuel Cells and Electrochemical Kinetics, and textbooks on Electrochemistry. From 1986 to 1993, Professor Vielstich was co-ordinator of the first European project on the DMFC and in 1998 he received the Faraday Medal of the Royal Chemical Society, UK.
Hubert A. Gasteiger received his Ph.D. in Chemical Engineering from the University of California at Berkeley in 1993, studying the electrocatalysis of methanol oxidation. After 9 years of academic research on fundamental electrocatalysis and heterogeneous gas-phase catalysis, he worked for 10 years in industrial R&D groups. From 1998 to 2007, Dr. Gasteiger was involved in the stack component design for GM/Opel's H2-powered fuel cell vehicles, leading an R&D group in MEA development and diagnostics at GM/Opel's Fuel Cell Activities program in Honeoye Falls, New York, where he was promoted to Technical Fellow in 2004. In 2007 he joined Acta S.p.A., Italy, as Director of Catalyst Technology , developing catalysts and electrodes for alkaline (membrane) fuel cells. In January 2009 he took an assignment as Visiting Professor at the Electrochemical Energy Lab in the Dept. of Mechanical Engineering at MIT.
He served as Co‑Editor-In-Chief for Wiley's Handbook of Fuel Cells - Fundamentals, Technology, and Applications (2003), and published 60 papers in refereed journals and 12 book chapters. In 2004, he received the Klaus-Jürgen Vetter Award for Electrochemical Kinetics from the International Society of Electrochemi
Harumi Yokokawa
1972 - Graduated from Nuclear Engineering department, University of Tokyo
1977 - Graduated from Doctor course of University of Tokyo
Title of Doctoral work "Calorimetric Investigation of Uranium Compounds"
1977 - Join to National Chemical Laboratory for Industry, Agency for Industrial Science and Technology, Ministry of International Trade and Industry (MITI)
1978-1980 - Research Associated in James Franck Institute, University of Chicago
1982 - Senior researcher, National Chemical Laboratory for Industry
1993 - National Institute of Materials and Chemical Research, AIST, MITI
2001 - National Institute of Advanced Industrial Science and Technology
Awards
1989 - Award by Japan Information Center for Science and Technology on "Construction of Thermodynamic database and its advanced utilization"
2001 - Award by Minister of Science and Technology Agency on "Construction of Thermodynamic database and its applications to energy related materials."
2002 - Outstanding Achievement Awards from the High Temperature Materials Divsion, The Electrochemical Society, Inc., "In recognition of his contributions to the practical applications of thermochemistry to high temperature materials research and technology, especially in the area of solid oxide fuel cells."
Table of Contents
| Contributors to Volume 5 and 6 |
| Foreword |
| Preface |
| Abbreviations and Acronyms |
| Part 1 Electrocatalyst Materials For Low Temperature Fuel Cells |
| Novel Catalysts |
| 1 Platinum monolayer oxygen reduction electrocatalystsR. R. Adzic and F. H. B. Lima |
| 2 Oxygen reduction on platinum bimetallic alloy catalystsV. R. Stamenkovic and N. M. Markovic |
| 3 Dealloyed Pt bimetallic electrocatalysts for oxygen reductionP. Strasser |
| 4 Transition metal/polymer catalysts for O2 reductionC. M. Johnston and P. Piela and P. Zelenay |
| 5 Time to move beyond transition metal-N-C catalysts for oxygen reductionA. Garsuch and A. Bonakdarpour and G. Liu and R. Yang and J. R. Dahn |
| 6 Catalysts for the electro-oxidation of small moleculesM. Watanabe and H. Uchida |
| 7 Influence of size on the electrocatalytic activities of supported metal nanoparticles in fuel cell-related reactionsFrédéric Maillard and Sergey Pronkin and Elena R. Savinova |
| 8 Enzyme catalysis in biological fuel cellsScott Calabrese Barton |
| Fundamental Catalysis Models |
| 9 Density functional theory applied to electrocatalysisS. Venkatachalam and T. Jacob |
| 10 First-principles modeling for the electrooxidation of small moleculesM. Neurock |
| 11 On the pathways of methanol and ethanol oxidationW. Vielstich and V. A. Paganin and O. Brandao Alves and E. G. Ciapina |
| 12 Reaction pathway analysis and reaction intermediate detection |
| via simultaneous differential electrochemical mass spectrometry |
| (DEMS) and attenuated total reflection fourier transform infrared spectroscopy (ATR-FTIRS)M. Heinen and Z. Jusys and R. J. Behm |
| 13 Methanol oxidation on oxidized Pt surfaceH. Varela and E. Sitta and B. C. Batista |
| 14 Mechanistic aspects of carbon monoxide oxidationT. Iwasita and E. G. Ciapina |
| Catalyst Durability |
| 15 Platinum dissolution models and voltage cycling effects: platinum dissolution in polymer electrolyte fuel cell (PEFC) and low-temperature fuel cellsK. Ota and Y. Koizumi |
| 16 Catalyst and catalyst-support durabilityF. T. Wagner and S. G. Yan and P. T. Yu |
| 17 Effects of contaminants on catalyst activityF. H. Garzon and F. A. Uribe |
| Part 2 Conductive Membranes For Lowtemperature Fuel Cells |
| Novel Materials |
| 18 Design rules for the improvement of the performance of hydrocarbon-based membranes for proton exchange membrane fuel cells (PEMFC)M. Gross and G. Maier and T. Fuller and S. MacKinnon and C. Gittleman |
| 19 High-temperature polybenzimidazole-based membranesD. C. Seel and B. C. Benicewicz and L. Xiao and T. J. Schmidt |
| 20 Radiation-grafted proton conducting membranesL. Gubler and G. G. Scherer |
| 21 Alkaline anion-exchange membranes for low-temperature fuel cell applicationJ. R. Varcoe and S. D. Poynton and R. C. T. Slade |
| Characterization |
| 22 Colloidal structure of ionomer solutionsG. Gebel |
| 23 Conductivity, permeability, and ohmic shorting of ionomeric membranesC. K. Mittelsteadt and H. Liu |
| Membrane Durability |
| 24 Highly durable PFSA membranesE. Endoh |
| 25 Factors influencing ionomer degradationM. Inaba and H. Yamada |
| 26 Chemical and mechanical membrane degradationW. K. Liu and S. J. C. Cleghorn and B. E. Delaney and M. Crum |
| 27 Mechanical durability characterization and modeling of ionomeric membranesY. H. Lai and D. A. Dillard |
| Part 3 Materials For High Temperature Fuel Cells |
| Fundamental Models |
| 28 Mechanistic understanding and electrochemical modeling of mixed conducting (SOFC) electrodesR. Merkle and J. Maier and J. Fleig |
| 29 Elementary kinetic modeling of solid oxide fuel cell electrode reactionsS. B. Adler and W. G. Bessler |
| 30 Mechanical stabilityA. Atkinson and A. J. Marquis |
| Novel Materials |
| 31 Factors limiting the low-temperature operation of SOFCsJ. David Carter and T. A. Cruse and B. J. Ingram and M. Krumpelt |
| 32 New oxide cathodes and anodesJ. A. Kilner and J. T. S. Irvine |
| 33 New high-temperature proton conductors for fuel cells and gas separation membranesR. Haugsrud |
| 34 Nanoimpact on electrode and electrolyte layers with Micro-Electro-Mechanical System (MEMS) techniqueY. D. Premchand and A. Bieberle-Hûtter and H. Galinski and J. L. M. Rupp and T. M. Ryll and B. Scherrer and R. Tölke and Z. Yang and A. Harvey and A. Evans and L. Xu and L. J. Gauckler |
| Materials Durability |
| 35 Durability of metallic interconnects and protective coatingsM. Mogensen and K. V. Hansen |
| 36 Impact of impurities and interface reaction on electrochemical activityM. Mogensen and K. V. Hansen |
| 37 Application of secondary ion mass spectrometry (SIMS) technique on the durability of solid oxide fuel cell (SOFC) materialsK. Yamaji and N. Sakai and H. Kishimoto and T. Horita and M. E. Brito and H. Yokokawa |
| 38 Durability of cathodes including Cr poisoningN. H. Menzler and A. Mai and D. Stöver |
| 39 Durable sealing concepts with glass sealants or compression sealsH. P. Buchkremer and R. Conradt |
| Part 4 Advanced Diagnostics, Models, & Design |
| Low-Temperature Fuel Cells |
| 40 Direct three-dimensional visualization and morphological analysis of Pt particles supported on carbon by transmission electron microtomographyT. Ito and U. Matsuwaki and Y. Otsuka and G. Katagiri and M. Kato and K. Matsubara and Y. Aoyama and H. Jinnai |
| 41 Design approaches for determining local current and membrane resistance in polymer electrolyte fuel cells (PEFCs)S. A. Freunberger and M. Reum and F. N. B?uchi |
| 42 Heat and water transport models for polymer electrolyte fuel cellsU. Pasaogullari |
| 43 Proton exchange membrane fuel cell (PEMFC) down-the-channel performance modelW. Gu and D. R. Baker and Y. Liu and H. A. Gasteiger |
| 44 Use of neutron imaging for proton exchange membrane fuel cell (PEMFC) performance analysis and designT. A. Trabold and J. P. Owejan and J. J. Gagliardo and D. L. Jacobson and D. S. Hussey and M. Arif |
| 45 Local transient techniques in polymer electrolyte fuel cell (PEFC) diagnosticsI. A. Schneider and G. G. Scherer |
| 46 Proton exchange membrane fuel cell (PEMFC) flow-field design for improved water managementJ. S. Allen and S. Y. Son and S. H. Collicott |
| 47 Performance during start-up of proton exchange membrane (PEM) fuel cells at subfreezing conditionsE. L. Thompson and W. Gu and H. A. Gasteiger |
| 48 Performance impact of cationic contaminantsB. S. Pivovar and B. Kienitz and T. Rockward and F. Uribe and F. Garzon |
| 49 Modeling the impact of cation contamination in a polymer electrolyte membrane fuel cellT. A. Greszler and T. E. Moylan and H. A. Gasteiger |
| 50 Performance modeling and cell design for high concentration methanol fuel cellsC. E. Shaffer and C. Y. Wang |
| 51 Design concepts and durability challenges for mini fuel cellsShimshon Gottesfeld |
| High-Temperature Fuel Cells |
| 52 New diagnostic methods for the polarized stateT. Kawada |
| 53 Electrochemical impedance spectroscopy as diagnostic toolS. H. Jensen and J. Hjelm and A. Hagen and M. Mogensen |
| 54 Observation and modeling of thermal stresses in cells and cell stacksH. Yakabe |
| Part 5 Performance Degradation |
| Low-Temperature Fuel Cells |
| 55 Carbon-support corrosion mechanisms and modelsK. G. Gallagher and R. M. Darling and T. F. Fuller |
| 56 Electrode degradation mechanisms studies by current distribution measurementsR. N. Carter and W. Gu and B. Brady and P. T. Yu and K. Subramanian and H. A. Gasteiger |
| 57 Electron microscopy to study membrane electrode assembly (MEA) materials and structure degradationM. Chatenet and L. Guetaz and F. Maillard |
| 58 Proton exchange membrane fuel cell degradation: mechanisms and recent progressT. Madden and M. Perry and L. Protsailo and M. Gummalla and S. Burlatsky and N. Cipollini and S. Motupally and T. Jarvi |
| 59 Cold-start durability of membrane-electrode assembliesC. Y. Wang and X. G. Yang and Y. Tabuchi and F. Kagami |
| 60 Field experience with fuel cell vehiclesK. Wipke and S. Sprik and J. Kurtz and J. Garbak |
| 61 Membrane and catalyst performance targets for automotive fuel cellsA. Iiyama and K. Shinohara and S. Iguchi and A. Daimaru |
| 62 Field experience with portable DMFC productsJ. Mûller |
| High-Temperature Fuel Cells |
| 63 Overview of solid oxide fuel cell degradationH. Yokokawa |
| 64 Methane reforming kinetics, carbon deposition, and redox durability of Ni/8 yttria-stabilized zirconia (YSZ) anodesE. Ivers-Tiffée and H. Timmermann and A. Leonide and N. H. Menzler and J. Malzbender |
| 65 Sulfur poisoning on Ni catalyst and anodesJ. B?gild Hansen and J. Rostrup-Nielsen |
| 66 Ni shorting in relation to acid-base equilibrium of molten carbonate for molten cabonate fuel cell (MCFC) applicationS. Mitsushima |
| 67 Impact of impurities on reliability of materials in solid oxide fuel cell (SOFC) stack/modulesH. Yokokawa and N. Sakai and T. Horita and K. Yamaji |
| 68 Field experience with molten carbonate fuel cells (MCFCs) and solid oxide fuel cells (SOFCs) with an emphasis on degradationH. Frey and A. Kessler and W. Mûnch and M. Edel and V. Nerlich |
| Subject Index |
